TAU Nanocenter

We predict a new universal pseudospin localization phenomenon and demonstrate it experimentally in an optical analogue of a spin-glass material - a disordered sum-frequency generation process in a nonlinear photonic crystal.

A new wave guiding mechanism is theoretically and experimentally demonstrated, using sum frequency generation and 2D periodically poled KTP crystals, where a frequency superposition beam is guided and manipulated on-chip without any linear refractive index change.

We predict a new universal pseudospin localization phenomenon and demonstrate it experimentally in an optical analogue of a spin-glass material–a disordered sum-frequency generation process in a nonlinear photonic crystal.

Tissue engineering is considered a promising approach to treating advanced degenerative maculopathies such as nonexudative age-related macular degeneration (AMD), the leading cause of blindness worldwide. The retina consists of several hierarchical tissue layers, each of which is supported by a layer underneath. Each of these layers has a different morphology and requires distinct conditions for proper assembly. In fact, a prerequisite step for the assembly of each of these layers is the organization of the layer underneath. Advanced retinal degeneration includes degeneration of the other retina layers, including the choroid, the retinal pigmented epithelium (RPE), and the photoreceptors. Here, we report a step-by-step fabrication process of a three-layer retinalike structure. The process included the 3D printing of a choroid-like structure in an extracellular matrix (ECM) hydrogel, followed by deposition of the RPE monolayer. After the formation of the blood vessel–RPE interface, the photoreceptor cells were deposited to interact with the RPE layer. At the end of the fabrication process, each layer was characterized for its morphology and expression of specific markers, and the integration of the three-layer retina was evaluated. We envision that such a retina-like structure may be able to attenuate the deterioration of a degenerated retina and improve engraftment and regeneration. This retinal implant may potentially be suitable for a spectrum of macular degenerative diseases for which there are currently no cures and may save millions from complete blindness.

A new waveguiding mechanism is theoretically and experimentally demonstrated, using sum frequency generation and 2D periodically poled KTP crystals, where a frequency superposition beam is guided and manipulated on-chip without any linear refractive index change.

Nanobubbles have been increasingly used in various applications involving porous media, such as groundwater remediation and irrigation. However, the fundamental scientific knowledge regarding the interactions between nanobubbles and the media is still limited. The interactions can be repulsive, attractive, or inert, and can involve reversible or irreversible attachment as well as destructive mechanisms. Specifically, the stability and mobility of nanobubbles in porous media is expected to be dependent on the dynamic conditions and the physicochemical properties of the porous media, solutions, and nanobubbles themselves. In this study, we investigated how changes in solution chemistry (pH, ionic strength, and valence) and media characteristics (size and wettability) affect the size and concentration of nanobubbles under dynamic conditions using column experiments. Quartz crystal microbalance with …

In 1974, Stephen Hawking predicted that quantum effects in the proximity of a black hole lead to the emission of particles and black hole evaporation. At the very heart of this process lies a logarithmic phase singularity which leads to the Bose-Einstein statistics of Hawking radiation. An identical singularity appears in the elementary quantum system of the inverted harmonic oscillator. In this Letter we report the observation of the onset of this logarithmic phase singularity emerging at a horizon in phase space and giving rise to a Fermi-Dirac distribution. For this purpose, we utilize surface gravity water waves and freely propagate an appropriately tailored energy wave function of the inverted harmonic oscillator to reveal the phase space horizon and the intrinsic singularities. Due to the presence of an amplitude singularity in this system, the analogous quantities display a Fermi-Dirac rather than a Bose-Einstein …

Lightwaves can be split into two beams or two pulses, each comprising a frequency-bin superposition, in the presence of a nonlinear coupling gradient, representing the nonlinear optics analog of the celebrated Stern-Gerlach effect for atoms.

We demonstrate a compact and efficient rotation sensing mechanism that uses structured light and is enhanced by bright N00N states. It uses two opposite spiral phase plates that convert mechanical rotation to wavefront phase shifts.

The Smith–Purcell effect allows for coherent free-electron-driven compact light sources over the entire electromagnetic spectrum. Intriguing interaction regimes, with prospects for quantum optical applications, are expected when the driving free electron enters the sub-keV range, though this has until now remained an experimental challenge. Here, we demonstrate the Smith–Purcell light emission from UV to visible using engineerable, fabricated gratings with periodicities as low as 19?nm and with electron energies as low as 300?eV. Our findings constitute a major step toward broadband, highly tunable, on-chip light sources, observation of quantum recoil effects, and tunable EUV and x ray sources from swift electrons.

Groundwater contamination by widespread and persistent organic compounds requires extensive treatment efforts, for example by in-situ chemical oxidation (ISCO). In this study, we investigated ozone mass transfer and removal mechanisms of ozone-resistant monocyclic aromatic and non-aromatic compounds in a novel in-situ treatment method using ozone-permeable membranes as reactive barrier. Initial batch experiments confirmed fast depletion of ozone in presence of sub-stoichiometric benzoic acid (BA), in contrast to the non-aromatic 1,4-dioxane (DIOX), where ozone depleted much slower. Simulated in-situ membrane ozonation treatment of contaminated groundwater led to lower removal of 5 mg L−1 BA (52.7%) compared to DIOX (60.6%). Inhibited removal of BA compared to additional batch experiments could be explained by quick depletion of ozone by reactive intermediates on the membrane surface …

Control over the joint spectral amplitude of a photon pair has proved highly desirable for many quantum applications, since it contains the spectral quantum correlations, and has crucial effects on the indistinguishability of photons, as well as promising emerging applications involving complex quantum functions and frequency encoding of qudits. Until today, this has been achieved by engineering a single degree of freedom, either by custom poling nonlinear crystal or by shaping the pump pulse. We present a combined approach where two degrees of freedom, the phase-matching function, and the pump spectrum, are controlled. This approach enables the two-dimensional control of the joint spectral amplitude, generating a variety of spectrally encoded quantum states - including frequency uncorrelated states, frequency-bin Bell states, and biphoton qudit states. In addition, the joint spectral amplitude is controlled …

The Stern-Gerlach experiment, a seminal quantum physics experiment, demonstrated the intriguing phenomenon of particle spin quantization, leading to applications in matter-wave interferometry and weak-value measurements. Over the years, several optical experiments have exhibited similar behavior to the Stern-Gerlach experiment, revealing splitting in both spatial and angular domains. Here we show, theoretically and experimentally, that the Stern-Gerlach effect can be extended into the time and frequency domains. By harnessing Kerr nonlinearity in optical fibers, we couple signal and idler pulses using two pump pulses, resulting in the emergence of two distinct eigenstates whereby the signal and idler are either in phase or out of phase. This nonlinear coupling emulates a synthetic magnetization, and by varying it linearly in time, one eigenstate deflects towards a higher frequency, while the other deflects …

The Stern-Gerlach experiment, a seminal quantum physics experiment, demonstrated the intriguing phenomenon of particle spin quantization, leading to applications in matter-wave interferometry and weak-value measurements. Over the years, several optical experiments have exhibited similar behavior to the Stern-Gerlach experiment, revealing splitting in both spatial and angular domains. Here we show, theoretically and experimentally, that the Stern-Gerlach effect can be extended into the time and frequency domains. By harnessing Kerr nonlinearity in optical fibers, we couple signal and idler pulses using two pump pulses, resulting in the emergence of two distinct eigenstates whereby the signal and idler are either in phase or out of phase. This nonlinear coupling emulates a synthetic magnetization, and by varying it linearly in time, one eigenstate deflects towards a higher frequency, while the other deflects …

Cavity quantum electrodynamics (QED), wherein a quantum emitter is coupled to electromagnetic cavity modes, is a powerful platform for implementing quantum sensors, memories, and networks. However, due to the fundamental tradeoff between gate fidelity and execution time, as well as limited scalability, the use of cavity-QED for quantum computation was overtaken by other architectures. Here, we introduce a new element into cavity-QED - a free charged particle, acting as a flying qubit. Using free electrons as a specific example, we demonstrate that our approach enables ultrafast, deterministic and universal discrete-variable quantum computation in a cavity-QED-based architecture, with potentially improved scalability. Our proposal hinges on a novel excitation blockade mechanism in a resonant interaction between a free-electron and a cavity polariton. This nonlinear interaction is faster by several orders of magnitude with respect to current photon-based cavity-QED gates, enjoys wide tunability and can demonstrate fidelities close to unity. Furthermore, our scheme is ubiquitous to any cavity nonlinearity, either due to light-matter coupling as in the Jaynes-Cummings model or due to photon-photon interactions as in a Kerr-type many-body system. In addition to promising advancements in cavity-QED quantum computation, our approach paves the way towards ultrafast and deterministic generation of highly-entangled photonic graph states and is applicable to other quantum technologies involving cavity-QED.

Cavity QED, wherein a quantum emitter is coupled to electromagnetic cavity modes, is a powerful platform for implementing quantum sensors, memories, and networks. However, due to the fundamental trade-off between gate fidelity and execution time, as well as limited scalability, the use of cavity QED for quantum computation was overtaken by other architectures. Here, we introduce a new element into cavity QED—a free charged particle, acting as a flying qubit. Using free electrons as a specific example, we demonstrate that our approach enables ultrafast, deterministic, and universal discrete-variable quantum computation in a cavity-QED-based architecture, with potentially improved scalability. Our proposal hinges on a novel excitation blockade mechanism in a resonant interaction between a free-electron and a cavity polariton. This nonlinear interaction is faster by several orders of magnitude with respect to …

More than three decades after the inception of electron spin-based information encoding inspired by nonlinear electro-optic devices, we present a complementary approach: nonlinear optical devices directly inspired by spintronics. We theoretically propose an all-optical spin-valve device and a spin-dependent beam splitter, where the optical pseudospin is a superposition of signal and idler beams undergoing a sum-frequency generation process inside a 2D nonlinear photonic crystal. We delve into the operation of these devices, examining key properties such as the transmission angle and splitting ratio, optically controlled by the pump beam. Our findings open new avenues for both classical and quantum optical information processing in the frequency domain.

This study demonstrates the use of a MnO2-coated gas-permeable membrane for efficient radical delivery to water. MnO2 of various morphologies─including nanowires (NW), nanosheets (NS) and nanoflowers (NF)─were synthesized, characterized, and evaluated according to their catalytic ozonation. In the presence of dissolved ozone, all forms of suspended MnO2 resulted in elevated hydroxyl radical exposure but still differed across morphologies. MnO2 NS resulted in a more efficient catalytic ozonation per mass and was thus synthesized on gas-permeable membrane tubes as a proof-of-concept. Polydimethylsiloxane (PDMS) membrane tubing was used as a platform, as it has been shown to enable effective passive diffusion of ozone driven by concentration gradients. The coated membrane allowed direct hydroxyl radical generation in a two-step process. First, the gaseous ozone passes through the inner …

This study demonstrates the use of a MnO2-coated gas-permeable membrane for efficient radical delivery to water. MnO2 of various morphologies─including nanowires (NW), nanosheets (NS) and nanoflowers (NF)─were synthesized, characterized, and evaluated according to their catalytic ozonation. In the presence of dissolved ozone, all forms of suspended MnO2 resulted in elevated hydroxyl radical exposure but still differed across morphologies. MnO2 NS resulted in a more efficient catalytic ozonation per mass and was thus synthesized on gas-permeable membrane tubes as a proof-of-concept. Polydimethylsiloxane (PDMS) membrane tubing was used as a platform, as it has been shown to enable effective passive diffusion of ozone driven by concentration gradients. The coated membrane allowed direct hydroxyl radical generation in a two-step process. First, the gaseous ozone passes through the inner …

More than three decades after the inception of electron spin-based information encoding inspired by nonlinear electro-optic devices, we present a complementary approach: nonlinear optical devices directly inspired by spintronics. We theoretically propose an all-optical spin-valve device and a spin-dependent beam splitter, where the optical pseudospin is a superposition of signal and idler beams undergoing a sum-frequency generation process inside a 2D nonlinear photonic crystal. We delve into the operation of these devices, examining key properties such as the transmission angle and splitting ratio, optically controlled by the pump beam. Our findings open new avenues for both classical and quantum optical information processing in the frequency domain.

Cardiac monitoring after heart surgeries is crucial for health maintenance and detecting postoperative complications early. However, current methods like rigid implants have limitations, as they require performing second complex surgeries for removal, increasing infection and inflammation risks, thus prompting research for improved sensing monitoring technologies. Herein, we introduce a nanosensor platform that is biodegradable, biocompatible, and integrated with multifunctions, suitable for use as implants for cardiac monitoring. The device has two electrochemical biosensors for sensing lactic acid and pH as well as a pressure sensor and a chemiresistor array for detecting volatile organic compounds. Its biocompatibility with myocytes has been tested in vitro, and its biodegradability and sensing function have been proven with ex vivo experiments using a three-dimensional (3D)-printed heart model and 3D …