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Jul 2023 • Results in Physics

Insecurity of a relativistic quantum commitment scheme

Guang Ping He

We propose a cheating strategy to a relativistic quantum commitment scheme (Nadeem, 2014) which was claimed to be unconditionally secure. It is shown that the sender Alice can cheat successfully with probability 100%, thus disproving the security claim.

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Jul 2023 • Physical Review B

Proximitized insulators from disordered superconductors

Moshe Haim, David Dentelski, Aviad Frydman

We present an experimental study of bilayers of a disordered Ag metal layer close to the metal-insulator transition and an indium-oxide film which is on the insulating side of the superconductor insulator transition. Our results show that superconducting fluctuations within the indium-oxide film, that proximitize the underlying metal layer, induce insulating rather than superconducting behavior. This is ascribed to suppression of density of states (due to the superconducting energy gap) for quasiparticles in the proximitized regions. Our results present a manifestation of the proximity effect phenomenon and provide important insight into the nature of the insulating phase of the disorder driven superconductor insulator transition.

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Jul 2023 • Laser & Photonics Reviews

Deep-Subwavelength Resonant Meta-Optics Enabled by Ultra-High Index Topological Insulators

Singh, D., Nandi, S., Fleger, Y., Cohen, S. Z., Lewi, T.

In nanophotonics, small mode volumes, high‐quality factor resonances, and large field enhancements without metals fundamentally scale with the refractive index and are key for many implementations involving light‐matter interactions. Topological insulators (TIs) are a class of insulating materials that host topologically protected surface states, some of which exhibit extraordinarily high permittivity values. Here, the optical properties of TI bismuth telluride (Bi2Te3) single crystals are studied. It is found that both the bulk and surface states contribute to the extremely large optical constants, with the real part of the refractive index peaking at n ≈ 11. Utilizing these ultra‐high index values, it is demonstrated that Bi2Te3 metasurfaces are capable of squeezing light in deep‐subwavelength structures, with the fundamental magnetic dipole (MD) resonance confined in unit cell sizes smaller than λ/10. It is further shown that …

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Jul 2023 • Nature Communications 14 (1), 1462, 2023

B cell class switch recombination is regulated by DYRK1A through MSH6 phosphorylation

Liat Stoler-Barak, Ethan Harris, Ayelet Peres, Hadas Hezroni, Mirela Kuka, Amalie Grenov, Neta Gurwicz, Meital Kupervaser, Bon Ham Yip, Matteo Iannacone, Gur Yaari, John Crispino, Ziv Shulman

B cell class switch recombination is regulated by DYRK1A through MSH6 phosphorylation | Research Square Research Square Browse Preprints COVID-19 Preprints Protocols Videos Journals Tools & Services Overview Digital Editing Professional Editing Badges Research Promotion Your Cart About Preprint Platform In Review Editorial Policies FAQ Our Team Advisory Board Blog Sign In Submit a Preprint Cite Share Download PDF Article B cell class switch recombination is regulated by DYRK1A through MSH6 phosphorylation Liat Stoler-Barak, Ethan Harris, Ayelet Peres, Hadas Hezroni, and 9 more This is a preprint; it has not been peer reviewed by a journal. https://doi.org/10.21203/rs.3.rs-1779641/v1 This work is licensed under a CC BY 4.0 License Status: Under Review Nature Portfolio Version 1 posted 05 Jul, 2022 You are reading this latest preprint version Abstract Protection from viral infections depends …

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Jul 2023 • Electrochimica Acta

First isolation of solvated MgCl+ species as the sole cations in electrolyte solutions for rechargeable Mg batteries

Ananya Maddegalla, Yogendra Kumar, Sankalpita Chakrabarty, Yuri Glagovsky, Bruria Schmerling, Natalia Fridman, Michal Afri, Hagit Aviv, Doron Aurbach, Ayan Mukherjee, Dmitry Bravo-Zhivotovskii, Malachi Noked

Synthesis of complex magnesium cations in ethereal solutions, is receiving a lot of attention due to their potential utilization in rechargeable magnesium batteries (RMB). The simplest complex cation, namely, solvated MgCl+, was hypothesized and reported as the most important cation in nonaqueous magnesium electrolyte solutions chemistry. However, such ions have never been isolated as the only cationic species in ethereal solutions developed for RMB. In this study, we report on successful isolation of the pure electrolyte MgCl(THF)5+ - PhAlCl3−, and on the electrochemical behavior of it in ethereal solutions. The structure of this compound was proved by single-crystal X-ray diffraction, Raman, and NMR spectroscopies. The novel MgCl(THF)5PhAlCl3/THF electrolyte solutions exhibit reversible Mg deposition/dissolution processes with anodic stability up to 2.7 V. The application of electrochemical cleaning pre …

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Jul 2023 • ACS Applied Nano Materials

Metal Nanoparticle/Photosystem I Protein Hybrids Coupled to Microantenna Afford Biologically and Electronically Controlled Localized Surface Plasmon Resonance: Implications for …

Itai Carmeli, Ibrahim Tanriover, Tirupathi Malavath, Chanoch Carmeli, Moshik Cohen, Yossi Abulafia, Olga Girshevitz, Shachar Richter, Koray Aydin, Zeev Zalevsky

Localized surface plasmon resonance (LSPR) holds great promise for the next generation of fast nanoscale optoelectronic devices, as silicon-based electronic devices approach fundamental speed and scaling limitations. However, in order to fully exploit the potential of plasmonics, devices and material systems capable of actively controlling and manipulating plasmonic response are essential. Here, we demonstrate active control of the electric field distribution of a microantenna by coupling LSPRs to a photosynthetic protein with outstanding optoelectronic properties and a long-range and efficient exciton transfer ability. The hybrid biosolid state active platform is able to tune and modulate the optical activity of a microplasmonic antenna via the interaction of the bioactive material with plasmon oscillations occurring in the antennae. In addition, we demonstrate that the effect of the coupling can be further enhanced …

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Jul 2023 • Cells

Propofol inhibits glioma stem cell growth and migration and their interaction with microglia via BDNF-AS and extracellular vesicles

Rephael Nizar, Simona Cazacu, Cunli Xiang, Matan Krasner, Efrat Barbiro-Michaely, Doron Gerber, Jonathan Schwartz, Iris Fried, Shira Yuval, Aharon Brodie, Gila Kazimirsky, Naama Amos, Ron Unger, Stephen Brown, Lisa Rogers, Donald H Penning, Chaya Brodie


Jul 2023 • arXiv preprint arXiv:2307.01874

Non-relativistic spatiotemporal quantum reference frames

Michael Suleymanov, Ismael L Paiva, Eliahu Cohen

Quantum reference frames have attracted renewed interest recently, as their exploration is relevant and instructive in many areas of quantum theory. Among the different types, position and time reference frames have captivated special attention. Here, we introduce and analyze a non-relativistic framework in which each system contains an internal clock, in addition to its external (spatial) degree of freedom and, hence, can be used as a spatiotemporal quantum reference frame. Among other applications of this framework, we show that even in simple scenarios with no interactions, the relative uncertainty between clocks affects the relative spatial spread of the systems.

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Jul 2023 • ACS Applied Nano Materials

Metal Nanoparticle/Photosystem I Protein Hybrids Coupled to Microantenna Afford Biologically and Electronically Controlled Localized Surface Plasmon Resonance: Implications for …

Itai Carmeli, Ibrahim Tanriover, Tirupathi Malavath, Chanoch Carmeli, Moshik Cohen, Yossi Abulafia, Olga Girshevitz, Shachar Richter, Koray Aydin, Zeev Zalevsky

Localized surface plasmon resonance (LSPR) holds great promise for the next generation of fast nanoscale optoelectronic devices, as silicon-based electronic devices approach fundamental speed and scaling limitations. However, in order to fully exploit the potential of plasmonics, devices and material systems capable of actively controlling and manipulating plasmonic response are essential. Here, we demonstrate active control of the electric field distribution of a microantenna by coupling LSPRs to a photosynthetic protein with outstanding optoelectronic properties and a long-range and efficient exciton transfer ability. The hybrid biosolid state active platform is able to tune and modulate the optical activity of a microplasmonic antenna via the interaction of the bioactive material with plasmon oscillations occurring in the antennae. In addition, we demonstrate that the effect of the coupling can be further enhanced …

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Jul 2023 • APL Photonics

Opto-mechanical fiber sensing with optical and acoustic cladding modes

Avi Zadok, Elad Zehavi, Alon Bernstein

Optical fibers are an excellent sensor platform. However, the detection and analysis of media outside the cladding and coating of standard fibers represent a long-standing challenge: light that is guided in the single optical core mode does not reach these media. Cladding modes help work around this difficulty, as their transverse profiles span the entire cross-section of the fiber cladding and reach its outer boundary. In this tutorial, we introduce and discuss in detail two recent advances in optical fiber sensors that make use of cladding modes. Both concepts share optomechanics as a common underlying theme. First, we describe a spatially continuous distributed analysis using the optical cladding modes of the fiber. Light is coupled to these modes using Brillouin dynamic gratings, which are index perturbations associated with acoustic waves in the core that are stimulated by light. Unlike permanent gratings, which …

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Jul 2023 • Electrochimica Acta

First isolation of solvated MgCl+ species as the sole cations in electrolyte solutions for rechargeable Mg batteries

Ananya Maddegalla, Yogendra Kumar, Sankalpita Chakrabarty, Yuri Glagovsky, Bruria Schmerling, Natalia Fridman, Michal Afri, Hagit Aviv, Doron Aurbach, Ayan Mukherjee, Dmitry Bravo-Zhivotovskii, Malachi Noked

Synthesis of complex magnesium cations in ethereal solutions, is receiving a lot of attention due to their potential utilization in rechargeable magnesium batteries (RMB). The simplest complex cation, namely, solvated MgCl+, was hypothesized and reported as the most important cation in nonaqueous magnesium electrolyte solutions chemistry. However, such ions have never been isolated as the only cationic species in ethereal solutions developed for RMB. In this study, we report on successful isolation of the pure electrolyte MgCl(THF)5+ - PhAlCl3−, and on the electrochemical behavior of it in ethereal solutions. The structure of this compound was proved by single-crystal X-ray diffraction, Raman, and NMR spectroscopies. The novel MgCl(THF)5PhAlCl3/THF electrolyte solutions exhibit reversible Mg deposition/dissolution processes with anodic stability up to 2.7 V. The application of electrochemical cleaning pre …

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Jul 2023 • Nanomaterials

Probing Polarity and pH Sensitivity of Carbon Dots in Escherichia coli through Time-Resolved Fluorescence Analyses

Gilad Yahav, Shweta Pawar, Anat Lipovsky, Akanksha Gupta, Aharon Gedanken, Hamootal Duadi, Dror Fixler

Intracellular monitoring of pH and polarity is crucial for understanding cellular processes and functions. This study employed pH- and polarity-sensitive nanomaterials such as carbon dots (CDs) for the intracellular sensing of pH, polarity, and viscosity using integrated time-resolved fluorescence anisotropy (FA) imaging (TR-FAIM) and fluorescence lifetime (FLT) imaging microscopy (FLIM), thereby enabling comprehensive characterization. The functional groups on the surface of CDs exhibit sensitivity to changes in the microenvironment, leading to variations in fluorescence intensity (FI) and FLT according to pH and polarity. The FLT of CDs in aqueous solution changed gradually from 6.38 ± 0.05 ns to 8.03 ± 0.21 ns within a pH range of 2–8. Interestingly, a complex relationship of FI and FLT was observed during measurements of CDs with decreasing polarity. However, the FA and rotational correlation time (θ) increased from 0.062 ± 0.019 to 0.112 ± 0.023 and from 0.49 ± 0.03 ns to 2.01 ± 0.27 ns, respectively. This increase in FA and θ was attributed to the higher viscosity accompanying the decrease in polarity. Furthermore, CDs were found to bind to three locations in Escherichia coli: the cell wall, inner membrane, and cytoplasm, enabling intracellular characterization using FI and FA decay imaging. FLT provided insights into cytoplasmic pH (7.67 ± 0.48), which agreed with previous works, as well as the decrease in polarity in the cell wall and inner membrane. The CD aggregation was suspected in certain areas based on FA, and the θ provided information on cytoplasmic heterogeneity due to the aggregation and/or interactions with …

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Jul 2023 • Optics Express

Split-well resonant-phonon terahertz quantum cascade laser

Shiran Levy, Nathalie Lander Gower, Silvia Piperno, Sadhvikas J Addamane, John L Reno, Asaf Albo

We present a highly diagonal “split-well resonant-phonon” (SWRP) active region design for GaAs/Al_0.3Ga_0.7As terahertz quantum cascade lasers (THz-QCLs). Negative differential resistance is observed at room temperature, which indicates the suppression of thermally activated leakage channels. The overlap between the doped region and the active level states is reduced relative to that of the split-well direct-phonon (SWDP) design. The energy gap between the lower laser level (LLL) and the injector is kept at 36 meV, enabling a fast depopulation of the LLL. Within this work, we investigated the temperature performance and potential of this structure.

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Jul 2023 • Nature Communications

A sodium-ion-conducted asymmetric electrolyzer to lower the operation voltage for direct seawater electrolysis

Hao Shi, Tanyuan Wang, Jianyun Liu, Weiwei Chen, Shenzhou Li, Jiashun Liang, Shuxia Liu, Xuan Liu, Zhao Cai, Chao Wang, Dong Su, Yunhui Huang, Lior Elbaz, Qing Li

Hydrogen produced from neutral seawater electrolysis faces many challenges including high energy consumption, the corrosion/side reactions caused by Cl-, and the blockage of active sites by Ca2+/Mg2+ precipitates. Herein, we design a pH-asymmetric electrolyzer with a Na+ exchange membrane for direct seawater electrolysis, which can simultaneously prevent Cl- corrosion and Ca2+/Mg2+ precipitation and harvest the chemical potentials between the different electrolytes to reduce the required voltage. In-situ Raman spectroscopy and density functional theory calculations reveal that water dissociation can be promoted with a catalyst based on atomically dispersed Pt anchored to Ni-Fe-P nanowires with a reduced energy barrier (by 0.26 eV), thus accelerating the hydrogen evolution kinetics in seawater. Consequently, the asymmetric electrolyzer exhibits current densities of 10 mA cm−2 and 100 mA cm …

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Jul 2023 • Electrochimica Acta

Advanced impedance analysis of direct quinone fuel cells using distribution of relaxation times

Yan Yurko, Lior Elbaz

The need for new, reliable, and sustainable energy sources led to the development of new types of fuel cells. Fuel cells that rely on liquid hydrogen carriers may be the ultimate solution to the expensive hydrogen logistics issues. In this category, direct quinone fuel cells (DQFCs) are a promising new technology that solves many of the issues of traditional fuel cells. As a new technology, DQFCs need to be studied thoroughly to reach their full potential. Here, we use a distribution of relaxation times (DRT) analysis to analyze the impedance data of DQFCs, to gain a better understanding of the system. We systematically changed the operating parameters and attributed the changes in the DRT spectra to the physical processes they correspond to. The four main peaks observed in the DRT measurements were assigned to oxygen reduction reaction (ORR), quinone diffusion resistance, proton diffusion in the membrane …

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Jul 2023 • 2023 23rd International Conference on Transparent Optical Networks (ICTON), 1-4, 2023

Microwave-Based Remote Bio-Sensing behind Walls

Ohad Meshulam, Nisan Ozana, Dan Scheffer, Shlomo Zach, Zeev Zalevsky

In this paper a novel method for microwave based remote sensing of vital signs behind walls is presented. The method is based on temporal spatial analysis of back scattered microwave signals. The use of non-optical electromagnetic radiation enables monitoring from larger distances and behind objects in contrast to similar concepts in optics. Further, such use of non-optical radiation omits the need for direct line of sight between the monitoring system and the target and enables monitoring through walls or other barriers. Micro-vibrations due to breathing and heart pulsation affect the reflection of microwaves and cause the self-interference random patterns (i.e. speckle patterns) to vary in time and space. By using this approach, the temporal change of the speckle patterns due to changes in vital signs can be tracked behind walls. In this paper we present a system in WiFi frequencies band consisting of two radio …

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Jul 2023 • 2023 Photonics & Electromagnetics Research Symposium (PIERS), 1275-1284, 2023

2D Mono Detection Spatially Super-resolved Microwave Imaging for Radar Applications

Isahar Gabay, Zeev Zalevsky

In this paper we present an advanced 2D novel microwave photonic approach to super resolved Radar imaging. Unlike synthetic aperture Radars (SAR) that require movement to improve resolution by synthetically increasing the antennas dimensions, our super resolved imaging solution not only does not require movement to synthetically increase the antennas dimensions but it also allows this super resolved sensing with only a single (mono) detector. The operation principle is based upon phased array antennas which consist of four radiating horn antennas which generate a projected plane at the far field zone. Setting an appropriate phase to each one of the antennas inputs, causes scanning of projected structured electromagnetic beam over the imaged object. Summing each azimuth cut of the reflections, received from the object at different frequencies can spatially reconstruct high resolution image of the …

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Jul 2023 • Electrochimica Acta

Simplified FTacV model to quantify the electrochemically active site density in PGM-free ORR catalysts

Ariel Friedman, Rifael Z Snitkoff-Sol, Hilah C Honig, Lior Elbaz

The development of platinum group metal-free catalysts is considered the most prominent path for reducing the cost of low-temperature fuel cells (LTFC). Despite the great advancement in the field, its further progress is currently limited by the ability to understand and mitigate the catalysts’ degradation mechanisms, which up to recent years was limited by the lack of activity descriptors. Recent work showed that this could be solved using Fourier-transformed alternating current voltammetry that enables to deconvolute Faradaic currents arising from the redox reaction of the active sites from the capacitive currents, and by that accurately measure the electrochemically active site density of these catalysts in situ fuel cells. However, the analysis of the results can be complex, requiring simulation software for accurate parameter extraction. Herein, a simplified analysis of Fourier-transformed alternating current voltammetry is …

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Jun 2023 • Electronic Structure

Multistate multiscale docking study of the hydrolysis of toxic nerve agents by phosphotriesterase

Prashant Kumar Gupta, Naziha Tarannam, Shani Levi, Dan Thomas Major

The G- and V-type nerve agents are among the most toxic compounds known, where inhalation of a few mg could cause potential death. Over the years, wild-type phosphotriesterase (PTE) has gained much attention due to its capability of detoxifying these deadly compounds. The underlying mechanism proceeds via a hydroxyl attack on the P or C centers of the organophosphate nerve agents, followed by the departure of the leaving group. Two Zn2+ cations present in the active center of PTE indirectly assist the hydrolysis. Apart from the wild-type PTE, several designer enzyme variants reportedly catalyze the hydrolysis process much more efficiently. Herein, we studied the hydrolysis of eight toxic compounds with one of the enzyme variants (PTE_27) that show higher efficiency than the wild type as reported in a recent article. We docked both the high energy intermediate state and substrate for all the eight ligands …

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Jun 2023 • NATURE

Magnetic memory and spontaneous vortices in a van der Waals superconductor (vol 607, pg 692, 2022)

Eylon Persky, Anders V Bjorlig, Irena Feldman, Avior Almoalem, Ehud Altman, Erez Berg, Itamar Kimchi, Jonathan Ruhman, Amit Kanigel, Beena Kalisky


Jun 2023 • Optics Continuum

Remote sensing of human skin temperature by AI speckle pattern analysis

Ofir Ben David, Yevgeny Beiderman, Sergey Agdarov, Yafim Beiderman, Zeev Zalevsky


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